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Articles

Año 9 No.26 Mayo - Agosto 2023

Atmospheric aerosols. Relevance in the planet's climate and a demonstrative experiment on its formation in the urban-forest interface

DOI
https://doi.org/10.32399/icuap.rdic.2448-5829.2023.26.1084
Submitted
May 22, 2023
Published
May 1, 2023

Abstract

Atmospheric aerosols are particles suspended in the atmosphere that vary in origin, size, and composition. In addition to being dangerous to human health, atmospheric aerosols can have short- and long-term effects on climate dynamics and are considered one of the greatest sources of uncertainty in global climate prediction models. In this work, we make an introduction to the subject of atmospheric aerosols as a key element of climate change. Likewise, a demonstrative experiment we carried out in the university laboratory is presented to illustrate one of the possible chemical mechanisms of aerosol formation from biogenic emissions from forests and secondary pollutants from cities, knowing that this type of chemical reaction occurs in the forest environment or at the forest-city interface. We consider it important to spread this phenomenon since forest ecosystems are basically considered particle sinks when particles are deposited on the surface of plants and leaves due to the mechanical effects of the wind. However, it is less known that forests can emit elements that are precursors to forming atmospheric aerosols. 

 

 

References

Andreae, M. O., & Crutzen, P. J. (1997). Atmospheric aerosols: Biogeochemical sources and role in atmospheric chemistry. Science, 276(5315), 1052–1058. https://doi.org/10.1126/science.276.5315.1052

Boelter, K. J., & Davidson, J. H. (1997). Ozone generation by indoor, electrostatic air cleaners. Aerosol Science and Technology, 27(6), 689–708. https://doi.org/10.1080/02786829708965505

Bréon, F. M., Tanré, D., & Generoso, S. (2002). Aerosol effect on cloud droplet size monitored from satellite. Science, 295(5556), 834–838. https://doi.org/10.1126/science.1066434

Che, H., Xia, X., Zhu, J., Wang, H., Wang, Y., Sun, J., … Shi, G. (2015). Aerosol optical properties under the condition of heavy haze over an urban site of Beijing, China. Environmental Science and Pollution Research, 22(2), 1043–1053. https://doi.org/10.1007/s11356-014-3415-5

Coleman, B. K., Lunden, M. M., Destaillats, H., & Nazaroff, W. W. (2008). Secondary organic aerosol from ozone-initiated reactions with terpene-rich household products. Atmospheric Environment, 42(35), 8234–8245. https://doi.org/10.1016/j.atmosenv.2008.07.031

Davidson, C. I., Phalen, R. F., & Solomon, P. A. (2005, August). Airborne particulate matter and human health: A review. Aerosol Science and Technology. https://doi.org/10.1080/02786820500191348

Ehara, K., Hagwood, C., & Coakley, K. J. (1996). Novel method to classify aerosol particles according to their mass-to-charge ratio - Aerosol particle mass analyser. Journal of Aerosol Science, 27(2), 217–234. https://doi.org/10.1016/0021-8502(95)00562-5

Gao, Y., Ma, M., Yan, F., Su, H., Wang, S., Liao, H., … Gao, H. (2022). Impacts of biogenic emissions from urban landscapes on summer ozone and secondary organic aerosol formation in megacities. Science of the Total Environment, 814, 152654. https://doi.org/10.1016/j.scitotenv.2021.152654

Hallquist, M., Wenger, J. C., Baltensperger, U., Rudich, Y., Simpson, D., Claeys, M., … Wildt, J. (2009). The formation, properties and impact of secondary organic aerosol: Current and emerging issues. Atmospheric Chemistry and Physics, 9(14), 5155–5236. https://doi.org/10.5194/acp-9-5155-2009

Haywood, J. (2016). Atmospheric Aerosols and Their Role in Climate Change. In Climate Change: Observed Impacts on Planet Earth: Second Edition (pp. 449–463). Elsevier Inc. https://doi.org/10.1016/B978-0-444-63524-2.00027-0

Houghton, J. T., Meira Filho, L. G., Callander, B. A., Harris, N. (Neil), Katternberg, A., Maskell, K. (Kathy), … WMO. (1996). Climate change 1995 :, 572. Retrieved from https://digitallibrary.un.org/record/223181

IPCC. (2013). Climate Change 2013: The Physical Science Basis. Working Group I Contribution to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change.

Jia, G. (2014). Atmospheric Residence Times of the Fine-aerosol in the Region of South Italy Estimated from the Activity Concentration Ratios of 210Po/210Pb in Air Particulates. Journal of Analytical & Bioanalytical Techniques, 5(6), 1–9. https://doi.org/10.4172/2155-9872.1000216

Lee, L. A., Reddington, C. L., & Carslaw, K. S. (2016). On the relationship between aerosol model uncertainty and radiative forcing uncertainty. Proceedings of the National Academy of Sciences of the United States of America, 113(21), 5820–5827. https://doi.org/10.1073/pnas.1507050113

Miller, R. L., & Tegen, I. (1998). Climate response to soil dust aerosols. Journal of Climate, 11(12), 3247–3267. https://doi.org/10.1175/1520-0442(1998)011<3247:CRTSDA>2.0.CO2

Pöschl, U. (2005, November 25). Atmospheric aerosols: Composition, transformation, climate and health effects. Angewandte Chemie - International Edition. https://doi.org/10.1002/anie.200501122

Ramanathan, V., Crutzen, P. J., Kiehl, J. T., & Rosenfeld, D. (2001). Aerosols, climate, and the hydrological cycle. Science (New York, N.Y.), 294(5549), 2119–2124. https://doi.org/10.1126/science.1064034

Riemer, N., & Ault, A. (2019). The Diversity and Complexity of Atmospheric Aerosol. Eos, 100. https://doi.org/10.1029/2019eo124333

Rodríguez, A., Andrés, V. S., Cervera, M., Redondo, A., Alquézar, B., Shimada, T., … Peña, L. (2011). The monoterpene limonene in orange peels attracts pests and microorganisms. Plant Signaling and Behavior, 6(11), 1820–1823. https://doi.org/10.4161/psb.6.11.16980

Seinfeld, J. H., & Pandis, S. N. (2016). Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, 3rd Edition | Wiley (3rd Editio). NY Wiley & Sons. Retrieved from https://www.wiley.com/en-us/Atmospheric+Chemistry+and+Physics%3A+From+Air+Pollution+to+Climate+Change%2C+3rd+Edition-p-9781118947401

Surratt, J. D., Murphy, S. M., Kroll, J. H., Ng, N. L., Hildebrandt, L., Sorooshian, A., … Seinfeld, J. H. (2006). Chemical composition of secondary organic aerosol formed from the photooxidation of isoprene. Journal of Physical Chemistry A, 110(31), 9665–9690. https://doi.org/10.1021/jp061734m

Yagi, S., & Tanaka, M. (1979). Mechanism of ozone generation in air-fed ozonisers. Journal of Physics D: Applied Physics, 12(9), 1509–1520. https://doi.org/10.1088/0022-3727/12/9/013